I have the eurorailpass and have problems using the app for bookings from Porto to Toledo or Madrid to Paris.
Solved
Train from Porto to Toledo; can't book reservations
Best answer by rvdborgt
Spain is very incomplete in the app because Spanish railways (RENFE) only share a part of their timetable with the rest of the world. For Spanish timetables, check the RENFE website or Rail Europe (who somehow managed to get timetables of Spanish long distance trains).
For the few connections that are left between Portugal and Spain, also check Seat61.
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